Build up of yield stress fluids via chaotic emulsification

Abstract
Stabilized dense emulsions display a rich phenomenology connecting microstructure and rheology. In this work we study how an emulsion with a finite yield stress can be built via large-scale stirring. By gradually increasing the volume fraction of the dispersed minority phase, under the constant action of a stirring force, we are able to achieve volume fractions close to 80%. Despite the fact that our system is highly concentrated and not yet turbulent we observe a droplet size distribution consistent with the -10/3 scaling, often associated to inertial range droplets breakup. We report that the polydispersity of droplet sizes correlates with the dynamics of the emulsion formation process. Additionally we quantify the visco-elastic properties of the dense emulsion finally obtained and we demonstrate the presence of a finite yield stress. The approach reported can pave the way to a quantitative understanding of the complex interplay between the dynamics of mesoscale constituents and the large scale flow properties yield-stress fluids.
Anno
2021
Tipo pubblicazione
Altri Autori
I. Girotto, R. Benzi, G. Di Staso, A. Scagliarini, F.S. Schifano, F. Toschi
Editore
American Physical Society
Rivista
Physical review research